Applied Chemical Engineering

  • Home
  • About
    • About the Journal
    • Article Processing Charges (APC) Payment
    • Contact
  • Articles
    • Current
    • Archives
  • Submissions
  • Editorial Team
  • Announcements
Register Login

Make a Submission

Make a Submission

editor-in-chief

Editors-in-Chief

Prof. Sivanesan Subramanian

Anna University, India

 

Prof. Hassan Karimi-Maleh

University of Electronic Science
and Technology of China (UESTC)

issn

ISSN

2578-2010 (Online)

indexing

 Indexing & Archiving 

 

 

 



Article Processing Charges

Article Processing Charges (APCs)

US$1600

publication_frequency

Publication Frequency

Quarterly

Keywords

Home > Archives > Vol. 9 No. 3(Publishing) > Original Research Article
ACE-6055

Published

2026-07-03

Issue

Vol. 9 No. 3(Publishing)

Section

Original Research Article

License

Copyright (c) 2026 Mo Li, Manus KAEWBUCHA, Chalisa APIWATHNASORN

Creative Commons License

This work is licensed under a Creative Commons Attribution 4.0 International License.

The Author(s) warrant that permission to publish the article has not been previously assigned elsewhere.

Author(s) shall retain the copyright of their work and grant the Journal/Publisher right for the first publication with the work simultaneously licensed under: 

 OA - Creative Commons Attribution-NonCommercial 4.0 International (CC BY-NC 4.0). This license allows for the copying, distribution and transmission of the work, provided the correct attribution of the original creator is stated. Adaptation and remixing are also permitted.

 

 This license intends to facilitate free access to, as well as the unrestricted reuse of, original works of all types for non-commercial purposes.

How to Cite

Mo Li, Manus KAEWBUCHA, & Chalisa APIWATHNASORN. (2026). Comparative Natural Dyeing and Bioactive Finishing of Cotton with Three Plant Extracts under FeSO₄ Fixation. Applied Chemical Engineering, 9(3), ACE-6055. https://doi.org/10.59429/ace.v9i3.6055
  • ACM
  • ACS
  • APA
  • ABNT
  • Chicago
  • Harvard
  • IEEE
  • MLA
  • Turabian
  • Vancouver

  • Download Citation
  • Endnote/Zotero/Mendeley (RIS)
  • BibTeX

Comparative Natural Dyeing and Bioactive Finishing of Cotton with Three Plant Extracts under FeSO₄ Fixation

Mo Li

Chakrabongse Bhuvanarth International College of Interdisciplinary Studies (CBIS), Rajamangala University of Technology Tawan-Ok, Bangkok, Thailand 10400

Manus KAEWBUCHA

Chakrabongse Bhuvanarth International College of Interdisciplinary Studies (CBIS), Rajamangala University of Technology Tawan-Ok, Bangkok, Thailand 10400

Chalisa APIWATHNASORN

Faculty of Fine and Applied Arts, Rajamangala University of Technology Thanyaburi, Khlong Luang, Pathum Thani, Thailand 12110


DOI: https://doi.org/10.59429/ace.v9i3.6055


Keywords: anthocyanins; plant polyphenols; eco-friendly coloration; mordanting; bioactive finishing; ultraviolet protection; antioxidant fabric; antibacterial textile


Abstract

Plant-derived colorants can combine textile coloration with bioactive finishing, but controlled comparisons among chemically distinct plant extracts on a common substrate remain limited. This study compared extracts from Lycium ruthenicum fruit, Broussonetia papyrifera fruit, and Rhodiola rosea root on a standardized plain-woven cotton substrate. Source-specific aqueous-ethanol extraction was followed by dyeing at an equal dry-extract concentration, and dyed fabrics were fixed with FeSO₄ for colour, fastness, and functional evaluation. Colour properties, washing/rubbing/light/perspiration fastness, ultraviolet protection factor (UPF), fabric antioxidant activity, and antibacterial activity against Staphylococcus aureus and Escherichia coli were evaluated. L. ruthenicum produced the deepest red-purple shade and the highest FeSO₄-assisted colour strength (K/S = 6.8), followed by B. papyrifera (4.6) and R. rosea(3.7). Under the common FeSO₄ fixation condition, the three extracts produced distinct colour and functional profiles, with L. ruthenicum showing the strongest overall performance. The antibacterial and antioxidant values represent the net response of the complete FeSO₄-fixed extract–cotton systems because separate extract-only and fixative-only controls were not included. These results support the potential of the tested plant sources for multifunctional cotton treatment while limiting the conclusions to the evaluated fixation route and initial performance conditions.


References

[1]. Al-Tohamy R, Ali SS, Li F, et al. A critical review on the treatment of dye-containing wastewater: ecotoxicological and health concerns of textile dyes and possible remediation approaches for environmental safety. Ecotoxicology and Environmental Safety 2022; 231: 113160. doi: 10.1016/j.ecoenv.2021.113160

[2]. Islam T, Repon MR, Islam T, et al. Impact of textile dyes on health and ecosystem: a review of structure, causes, and potential solutions. Environmental Science and Pollution Research 2023; 30: 9207–9242. doi: 10.1007/s11356-022-24398-3

[3]. Bhandari V, Badanayak P, Jose S. Plant-based colorants: isolation and application. In: Plant Biomass Derived Materials. Wiley; 2024. pp. 159–188. doi: 10.1002/9783527839032.ch7

[4]. Hamdy DM, Hassabo AG. Various natural dyes from different sources. Journal of Textiles, Coloration and Polymer Science 2021; 18(2): 171–190. doi: 10.21608/jtcps.2021.79786.1066

[5]. Islam S, Jalil MA, Belowar S, et al. Role of mordants in natural fabric dyeing and their environmental impacts. Environmental Science and Pollution Research 2025; 32: 452–468. doi: 10.1007/s11356-024-35746-w

[6]. Adeel S, Kiran S, Abbas M, et al. Sustainable isolation of licorice (Glycyrrhiza glabra L.)-based yellow natural colorant for dyeing of bio-mordanted cotton. Environmental Science and Pollution Research 2022; 29: 31270–31277. doi: 10.1007/s11356-021-18472-5

[7]. Liu Z, Tang X, Liu C, et al. Ultrasonic extraction of anthocyanins from Lycium ruthenicum Murr. and its antioxidant activity. Food Science & Nutrition 2020; 8(6): 2642–2651. doi: 10.1002/fsn3.1542

[8]. Islam T, Yu X, Badwal TS, Xu B. Comparative studies on phenolic profiles, antioxidant capacities and carotenoid contents of red goji berry (Lycium barbarum) and black goji berry (Lycium ruthenicum). Chemistry Central Journal 2017; 11: 59. doi: 10.1186/s13065-017-0287-z

[9]. Lee HS, Choi CI. Black goji berry (Lycium ruthenicum Murray): a review of its pharmacological activity. Nutrients 2023; 15(19): 4181. doi: 10.3390/nu15194181

[10]. Qin Y, Liu Y, Yong H, Liu J, Zhang X, Liu J. Preparation and characterization of active and intelligent packaging films based on cassava starch and anthocyanins from Lycium ruthenicum Murr. International Journal of Biological Macromolecules 2019; 134: 80–90. doi: 10.1016/j.ijbiomac.2019.05.029

[11]. Dong Y, Zhong W, Yang C, Zhang Y, Yang D. Study on anthocyanins from Lycium ruthenicum Murr via ultrasonic microwave synergistic extraction and its antioxidant properties. Frontiers in Sustainable Food Systems 2022; 6: 1052499. doi: 10.3389/fsufs.2022.1052499

[12]. Sun J, Liu SF, Zhang CS, et al. Chemical composition and antioxidant activities of Broussonetia papyrifera fruits. PLoS ONE 2012; 7(2): e32021. doi: 10.1371/journal.pone.0032021

[13]. Han Q, Wu Z, Huang B, et al. Extraction, antioxidant and antibacterial activities of Broussonetia papyrifera fruits polysaccharides. International Journal of Biological Macromolecules 2016; 92: 116–124. doi: 10.1016/j.ijbiomac.2016.06.087

[14]. Zhou XJ, Mei RQ, Zhang L, et al. Antioxidant phenolics from Broussonetia papyrifera fruits. Journal of Asian Natural Products Research 2010; 12(5): 399–406. doi: 10.1080/10286020.2010.481260

[15]. Li Y, Huang R, Zhang W, et al. Medicinal potential of Broussonetia papyrifera: chemical composition and biological activity analysis. Plants 2025; 14(4): 523. doi: 10.3390/plants14040523

[16]. Cao X, Yang L, Xue Q, et al. Antioxidant evaluation-guided chemical profiling and structure–activity analysis of leaf extracts from five trees in Broussonetia and Morus (Moraceae). Scientific Reports 2020; 10: 4808. doi: 10.1038/s41598-020-61709-5

[17]. Polumackanycz M, Konieczynski P, Orhan IE, Abaci N, Viapiana A. Chemical composition, antioxidant and anti-enzymatic activity of golden root (Rhodiola rosea L.) commercial samples. Antioxidants 2022; 11(5): 919. doi: 10.3390/antiox11050919

[18]. Dimpfel W, Schombert L, Panossian AG. Assessing the quality and potential efficacy of commercial extracts of Rhodiola rosea L. by analyzing the salidroside and rosavin content and the electrophysiological activity. Frontiers in Pharmacology 2018; 9: 425. doi: 10.3389/fphar.2018.00425

[19]. Tao H, Wu X, Cao J, et al. Rhodiola species: a comprehensive review of traditional use, phytochemistry, pharmacology, toxicity, and clinical study. Medicinal Research Reviews 2019; 39(5): 1779–1850. doi: 10.1002/med.21564

[20]. Cabral I. Ultraviolet-protective textiles: exploring the potential of cotton knits dyed with natural dyes. Textiles 2025; 5(3): 33. doi: 10.3390/textiles5030033

[21]. Gawish SM, Mashaly HM, Helmy HM, Ramadan AM, Farouk R. Effect of mordant on UV protection and antimicrobial activity of cotton, wool, silk and nylon fabrics dyed with some natural dyes. Journal of Nanomedicine & Nanotechnology 2017; 8: 421. doi: 10.4172/2157-7439.1000421

[22]. Singleton VL, Rossi JA. Colorimetry of total phenolics with phosphomolybdic-phosphotungstic acid reagents. American Journal of Enology and Viticulture 1965; 16: 144–158. doi: 10.5344/ajev.1965.16.3.144

[23]. Jia Z, Tang M, Wu J. The determination of flavonoid contents in mulberry and their scavenging effects on superoxide radicals. Food Chemistry 1999; 64(4): 555–559. doi: 10.1016/S0308-8146(98)00102-2

[24]. Lee J, Durst RW, Wrolstad RE. Determination of total monomeric anthocyanin pigment content of fruit juices, beverages, natural colorants, and wines by the pH differential method: collaborative study. Journal of AOAC International 2005; 88(5): 1269–1278. doi: 10.1093/jaoac/88.5.1269

[25]. Brand-Williams W, Cuvelier ME, Berset C. Use of a free radical method to evaluate antioxidant activity. LWT – Food Science and Technology 1995; 28(1): 25–30. doi: 10.1016/S0023-6438(95)80008-5

[26]. Re R, Pellegrini N, Proteggente A, Pannala A, Yang M, Rice-Evans C. Antioxidant activity applying an improved ABTS radical cation decolorization assay. Free Radical Biology and Medicine 1999; 26(9–10): 1231–1237. doi: 10.1016/S0891-5849(98)00315-3

[27]. Zhao Z, Hurren C, Zhang M, et al. In situ synthesis of a double-layer chitosan coating on cotton fabric to improve the color fastness of sodium copper chlorophyllin. Materials 2020; 13(23): 5365. doi: 10.3390/ma13235365

[28]. Mansour R, Ben Ali H. Investigating the use of chitosan: toward improving the dyeability of cotton fabrics dyed with Roselle (Hibiscus sabdariffa L.). Journal of Natural Fibers 2021; 18(7): 1007–1016. doi:10.1080/15440478.2019.1675217

[29]. Fang J, Meng C, Wang Y, et al. Eco-dyeing and functional finishing of cotton fabric by natural dye derived from lotus seedpod waste with chitosan-assistance. Fibers and Polymers 2023; 24(4): 1367–1377. doi: 10.1007/s12221-023-00158-z

[30]. Kubelka P, Munk F. Ein Beitrag zur Optik der Farbanstriche. Zeitschrift für technische Physik 1931; 12: 593–601.

[31]. Haji A, Shahmoradi Ghaheh F, Mohammadi L. Dyeing of polyamide 6 fabric with new bio-colorant and bio-mordants. Environmental Science and Pollution Research 2023; 30(13): 37981–37996. doi: 10.1007/s11356-022-24862-0

[32]. Hossain S, Jalil MA, Kader A, Kamal SA. Excellent dyeing properties of a natural dye extracted from the leaves of Phoenix dactylifera Linn on cotton and silk fabrics. Journal of Natural Fibers 2022; 19(15): 9803–9812. doi: 10.1080/00405000.2020.1763057

[33]. Hossain S, Jalil MA, Islam T, Mahmud RU, Kader A, Islam MK. Enhancement of antibacterial and UV protection properties of blended wool/acrylic and silk fabrics by dyeing with the extract of Mimusops elengi leaves and metal salts. Heliyon 2024; 10(3): e25273. doi: 10.1016/j.heliyon.2024.e25273

[34]. Zia KM, Adeel S, Aslam H, Khosa MK, Zuber M. Influence of ultrasonic radiation on extraction and green dyeing of mordanted cotton using neem bark extract. Journal of Industrial and Engineering Chemistry 2019; 77: 317–322. doi: 10.1016/j.jiec.2019.04.054

[35]. Banna BU, Mia R, Hasan MM, Ahmed B, Shibly MAH. Ultrasonic-assisted sustainable extraction and dyeing of organic cotton fabric using natural dyes from Dillenia indica leaf. Heliyon 2023; 9(8): e18702. doi: 10.1016/j.heliyon.2023.e18702

[36]. Hosseinnezhad M, Gharanjig K, Adeel S, Rouhani S, Imani H, Razani N. The effect of ultrasound on environmentally extraction and dyeing of wool yarns. Journal of Engineered Fibers and Fabrics 2022; 17: 1–10. doi: 10.1177/15589250221104471

[37]. Baig U, Khatri A, Ali S, et al. Ultrasound-assisted dyeing of cotton fabric with natural dye extracted from Marigold flower. Journal of the Textile Institute 2021; 112(5): 801–808. doi: 10.1080/00405000.2020.1779907

[38]. Jam N, Hajimohammadi R, Gharbani P, Mehrizad A. Evaluation of antibacterial activity of aqueous, ethanolic and methanolic extracts of areca nut fruit on selected bacteria. BioMed Research International 2021; 2021: 6663399. doi: 10.1155/2021/6663399.

[39]. Jam N, Hajimohammadi R, Gharbani P, Mehrizad A. Antibacterial activity of Punica granatum L. and areca nut (combined) extracts against some food borne pathogens. Saudi Journal of Biological Sciences 2022; 29(3): 1730–1736. doi: 10.1016/j.sjbs.2021.10.057.

[40]. Gharbani P, Jam N, Doshmanfekan H, Mehrizad A. Optimization of antibacterial activity of combined plant extracts by response surface methodology. Scientific Reports 2023; 13: 6098. doi: 10.1038/s41598-023-32900-1.

[41]. Gharbani P, Javazi H. The effect of developmental stage on antioxidant and biological activity of plant extract. Pakistan Journal of Pharmaceutical Sciences 2015; 28(5 Suppl): 1905–1909.

[42]. Tegegne W, et al. Natural dyeing and antibacterial finishing of cotton fabric with extracts from Justicia schimperiana leaf extract: a step towards sustainable dyeing and finishing. International Journal of Sustainable Engineering 2024; 17(1): 52–61. doi: 10.1080/19397038.2023.2301702

[43]. Muruganandham M, Tamilselvi Y, Sivasubramanian K, et al. Sustainable dyeing of cotton, silk and leather using natural dye from Bixa orellana seeds: extraction, optimization and assessment of antibacterial activity. Frontiers in Chemistry 2025; 13: 1474160. doi: 10.3389/fchem.2025.1474160

[44]. Nguyen TT, Nguyen TC, Nguyen TTT, Nguyen MH, Thai H. A comparative study on characteristics and antibacterial capacity of cotton fabrics dyed with reactive dye and Diospyros mollis extract. ChemistryOpen 2024; 13(11): e202400130. doi: 10.1002/open.202400130



ISSN: 2578-2010
21 Woodlands Close #02-10, Primz Bizhub,Postal 737854, Singapore

Email:editorial_office@as-pub.com